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Ultra-strong light–matter coupling for designer Reststrahlen band

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Ultra-strong light–matter coupling for designer Reststrahlen band
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The strength of the light–matter interaction depends on the number of dipoles that can couple with the photon trapped in an optical cavity. The coupling strength can thus be maximized by filling the entire cavity volume with an ensemble of interacting dipoles. In this work this is achieved by inserting a highly doped semiconductor layer in a subwavelength plasmonic resonator. In our system the ultra-strong light–matter coupling occurs between a collective electronic excitation and the cavity photon. The measured coupling strength is 73% of the matter excitation energy, the highest ever reported for a light–matter coupled system at room temperature. We experimentally and theoretically demonstrate that such an ultra-strong interaction modifies the optical properties on a very wide spectral range (20–250 meV), and results in the appearance of a photonic gap of 38 meV, independently of the light polarization and angle of incidence. Light–matter ultra-strong coupling can thus be exploited to conceive metasurfaces with an engineered reflectivity band.
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Transcript: English(auto-generated)
We are here at the Paris-Didro University, in the heart of Paris.
I'm Benjamin Askenazy, currently PhD student at the Laboratoire Materio et Phenomenes Contiques. In our team, we study quantum devices, operating from the mid-infrared to the terahertz regime. Those devices are based on inter-subband transition. They are designed and work with a picture of the electron behavior that can be described as a single particle.
In this paper, we go beyond this picture. Indeed, the usual picture of the inter-subband transition is the following. An electron stands on the lower level of the quantum well. A resonant photon can be absorbed, exciting the electron to the second level.
The electron can then re-emit the photon. This is the kind of picture used when designing quantum cascade lasers, for example. Now, if we increase the doping in the well, this single particle picture is no longer valid. The absorption spectrum will be blueshifted.
This is due to the fact that the electronic system must be seen as a collective excitation. An inter-subband plasmon. This is the well-known plasma shift. If we take a quantum well with several subbands occupied, a new system appears, the multi-subband plasmon. What's new with this structure is that despite several possible transitions,
the system only shows one absorption peak. Going further along this road, one could imagine reducing the energy separation between the subbands so much that the energy levels of the quantum well will tend towards a continuum. This is called a Behrmann mode, and once again, it shows only one absorption peak.
Now, this Behrmann mode has very interesting electronic properties for ultra-strong light-matter interaction. To demonstrate this, we put a Behrmann mode in an optical cavity. This cavity, called double-metal cavity, is made by two gold planes sandwiching a semiconductor layer.
One of the planes is patterned in squares to confine the light, as you can see on the cavity mode simulations. The Behrmann mode is then inserted in this cavity to interact with the trapped photons. The new states of the system, the so-called polaritons, are characterized by this dispersion.
The main point here is that those two curves are separated by a photonic gap. This is one of the characteristics of the ultra-strong coupling regime. The Rabi energy of the coupled system can be seen here. This gives us the strength of the light-matter interaction. 73% is the highest coupling ever reported for a room temperature system.
Now, this coupling strength can be used to design metamaterials with engineered band gaps. You can see here the optical index of bulk semiconductors in our cavities. There is a gap because of the phonons. Now, here is the optical index of our metamaterial.
We've added a gap which position and width can be adjusted. Thank you for watching this video abstract and enjoy your reading!