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Creating artificial photosystems

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Creating artificial photosystems
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29
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CC Attribution 4.0 International:
You are free to use, adapt and copy, distribute and transmit the work or content in adapted or unchanged form for any legal purpose as long as the work is attributed to the author in the manner specified by the author or licensor.
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Production Year2024
Production PlaceFrankfurt am Main

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Abstract
In nature, solar light energy conversion takes place within the thylakoid membrane during photosynthesis. Biomimetic lipid bilayers can be used as supramolecular scaffold to mimic concepts of photosynthesis to eventually generate fuels and high value chemicals using solar light as principal energy resource.[1,2] In the here presented work, lipid bilayer membranes of liposomes assemble chromophores for light harvesting energy transfer cascades, light induced transmembrane electron transfer, and (compartmentalized)[3] light driven conversions such as NADH conversion and CO2 reduction providing new directions for artificial photosynthesis and solar fuels generation. References [1] Pannwitz, A.; Klein, D. M.; Rodríguez-Jiménez, S.; Casadevall, C.; Song, H.; Reisner, E.; Hammarström, L.; Bonnet, S. Chem. Soc. Rev. 2021, 50, 4833–4855. [2] Sinambela, N.; Bösking, J.; Abbas, A.; Pannwitz, A ChemBioChem 2021, 22, 3140–3147. [3] Nau, R. E. P.; Bösking, J.; Pannwitz, A.; ChemPhotoChem 2022, 6, e202200158.
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